TAILORING THE ACTIVE SITE FOR THE OXYGEN EVOLUTION REACTION ON A PT ELECTRODE

Tailoring the active site for the oxygen evolution reaction on a Pt electrode

Tailoring the active site for the oxygen evolution reaction on a Pt electrode

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Accent Mug Electrocatalytic oxygen evolution is a key reaction for water splitting, but the detailed atomic structures of single-crystal electrodes under cycling conditions are still not fully understood.Here, the authors study the oxygen evolution activity on Pt(111) during potential cycling and find that the current density reaches a maximum in the third cycle and Gas Hob is nine times higher than that in the initial cycle, owing to a roughened Pt(111) surface and formation of islands and atomic vacancies in the second subsurface Pt layer.

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